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The quantum anomalous Hall effect refers to the quantization of the Hall effect in the absence of an applied magnetic field. The quantum anomalous Hall effect is of topological nature and well suited for field-free resistance metrology and low-power information processing utilizing dissipationless chiral edge transport. In this Perspective, we provide an overview of the recent achievements as well as the material challenges and opportunities, pertaining to engineering intrinsic/interfacial magnetic coupling, that are expected to propel future development in this field.more » « less
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Park, Eugene; Philbin, John_P; Chi, Hang; Sanchez, Joshua_J; Occhialini, Connor; Varnavides, Georgios; Curtis, Jonathan_B; Song, Zhigang; Klein, Julian; Thomsen, Joachim_D; et al (, Advanced Materials)Abstract The exploration of 1D magnetism, frequently portrayed as spin chains, constitutes an actively pursued research field that illuminates fundamental principles in many‐body problems and applications in magnonics and spintronics. The inherent reduction in dimensionality often leads to robust spin fluctuations, impacting magnetic ordering and resulting in novel magnetic phenomena. Here, structural, magnetic, and optical properties of highly anisotropic 2D van der Waals antiferromagnets that uniquely host spin chains are explored. First‐principle calculations reveal that the weakest interaction is interchain, leading to essentially 1D magnetic behavior in each layer. With the additional degree of freedom arising from its anisotropic structure, the structure is engineered by alloying, varying the 1D spin chain lengths using electron beam irradiation, or twisting for localized patterning, and spin textures are calculated, predicting robust stability of the antiferromagnetic ordering. Comparing with other spin chain magnets, these materials are anticipated to bring fresh perspectives on harvesting low‐dimensional magnetism.more » « less
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